If system 6 will even recognize that the above-2-gig volume is a real volume, there's no real telling what will happen.
The suggestion that it will "work but be erratic" comes from an Apple TIL/KB article about system 7.5.2, which was massively buggy and horrifically crashy, compared even to the "it's just a regular day on a Mac" level of crashiness that you might see using Mac OS 1-9.
I do know (having done this last year) a partition larger than 2GB System 7 will make the system act funny. Not going through every step, I will summarize the following:
- Using a 8GB CF on PCMCIA adapter, I partitioned it for 4GB partitions then 2.5GB partitions, and then 2GB partitions. It was able to format and give a Disk icon on the larger partitions but it could not could not write a system to it. It gave a "unable to rite file" error. I put the CF onto a OSX machine and put some files on it and it copied fine. Put it back in the 190, the file were there, but could not read them though the file icons were visible. And the amount of free Space was some odd low number on top of everything.
- Using the 2GB partition cleared things up. Files read and wrote, partitions formatted, free space showed up properly. Best of all a system installed and it booted.
- The idea was to format the CF in the PCMCIA and make it usable for a 1400cs with a dead hard drive. Switching Start Up Disk, and the 190 booted off the CF. Putting the CF into the 1400's IDE Port and it booted. No problems since. Later on I repartitioned it for 4GB and OS8.1 and it still works fine. But for System 6 and 7... the max is 2GB.
I think what he wants to know is the limit for the physical drive to be recognized by the system. That's a good question.
The SCSI of that era should be 24-bit LBA, if I'm not mistaken, so that's a hard limit for 8.4 GB.
If you put a larger drive in, the system will probably physically not recognize it.
That is an interesting question.
Because I stayed within those 2GB/4GB partition boundaries, the largest drives I ever put in a 68K Mac is a 8GB, I would not know how big of a drive can you put in. It's strange because I seen posts of "my hard drive died, can I use a 500GB replacement?" and when they do, the drive is dead to them. In some other cases, like in a smaller drive of 50GB, it works, sometimes.
For me, I figure - how big is the 68K (and later PowerPC) Mac Software Library? A couple of gigs? Of that, how big is my Mac Library? Less than 240MB. So why would anyone need a couple hundred gigs or even a tetrabyte of space for their Old Mac Software Library? Or their Multi-Media Library? 4 - 8 GB, I can see as a reasonable size for an old Mac System. But that is my opinion.